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OCR for page 191
Cleaning Up Sites Contaminated with Radioactive Materials: International Workshop Proceedings
24
Areas of the Russian Federation Affected by Radiation Contamination Due to the Chernobyl Nuclear Power Plant Accident*
S. M. Vakulovsky, T. S. Borodina, A. A. Volokitin, V. M. Kim, G. I. Petrenko, E. G. Tertyshnik, A. D. Uvarov, and V. N. Yakhryushin, Typhoon Research and Production Association—State Institution, Obninsk
As a result of the accident at the Chernobyl Nuclear Power Plant on April 26, 1986, 19 Russian Federation subjects (oblasts and autonomous republics) suffered cesium-137 contamination at levels of more than 1 Ci/km2 (37 kBq/m2). The total land area with this level of contamination in all the affected regions in 1986 was 65,050 km2. Table 24-1 presents a 1998 forecast of expected changes in the contamination level over time due to radioactive decay.1 As the table indicates, by 2006 the contaminated land area totaled 31,120 km2—that is, it had been reduced in size by one-half during the 20 years since the accident.
All population centers located in areas with cesium-137 contamination levels of more than 1 Ci/km2 (37 kBq/m2) were studied to determine their level of radiation contamination.2 The results of this research are presented in Table 24-2. From this table, it is clear that based on conditions in early 2006, there were 3,234 population centers in 15 Russian regions with cesium-137 contamination levels of more than 1 Ci/km2 (37 kBq/m2). For all these population centers, calcula-
*
Translated from the Russian by Kelly Robbins.
1
Izrael, Yu. A., et al. 1998. Long-term forecast of changes in the levels of Cs-137 radioactive contamination in areas of Russia after the Chernobyl Nuclear Power Plant accident. Meteorology and Hydrology 4:5-17.
2
The term population center encompasses urbanized areas of various sizes ranging from large cities to towns, villages, and small rural settlements.
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Cleaning Up Sites Contaminated with Radioactive Materials: International Workshop Proceedings
TABLE 24-1 Forecast of Expected Changes in Total Land Area in Russia with Varying Levels of Cesium-137 Radioactive Contamination Due to the Chernobyl Accident
Year
Area (in km2) with Varying Levels of Local Cs-137 Contamination
>40 Ci/km2
15-20 Ci/km2
5-15 Ci/km2
1-5 Ci/km2
1986
580
2,070
5,780
56,260
1996
310
1,900
5,330
48,980
2006
40
1,280
3,540
26,260
2016
850
2,780
18,920
2026
625
2,700
15,040
2036
190
2,340
12,500
2046
100
1,500
10,930
tions were made to determine how long it would take for each to move to the next lowest contamination category as a result of radioactive decay. The results of these calculations are presented in Table 24-3, which indicates that there will be no population centers with contamination levels greater than 40 Ci/km2 (1,480 kBq/m2) by 2020, greater than 15 Ci/km2 (555 kBq/m2) by 2063, greater than 5 Ci/km2 (185 kBq/m2) by 2110, and greater than 1 Ci/Km2 (37 kBq/m2) by 2180.
Bryansk Oblast suffered the most contamination from the Chernobyl accident of any Russian region. Therefore, information was compiled on the contamination status of the near-earth atmosphere (up to approximately 5 km from the earth’s surface) and bodies of water in this particular oblast. Figure 24-1 provides information on the change in the average annual cesium-137 activity by volume in the near-earth atmosphere over the city of Bryansk. From this figure, it is clear that the activity by volume decreased by an order of magnitude from 1987 to 1995. During the next 10 years, it changed insignificantly, fluctuating within the range of 1-3 × 10−6 Bq/m3. This amount is seven orders of magnitude lower than the activity by volume allowable for the population, as established by the Radiation Safety Norms (RSN-99).3 Levels of cesium-137 atmospheric fallout are cited for the population center of Krasnaya Gora (Figure 24-2), where the level of cesium-137 contamination is close to 5 Ci/km2 (185 kBq/m2), while near this town there is an area with substantially higher levels of soil contamination. Figure 24-2 shows that the level of atmospheric fallout declined by two orders of magnitude in the 5 years following 1986, changed insignificantly from 1991 through 2001, and subsequently fell to five times less by 2005. Figure 24-3 indicates that cesium-137 concentrations in the soil due to atmospheric fallout over 19 years totaled 11.5 kBq/m2, which is 6.2 percent of initial contamination.
3
Ministry of Health of the Russian Federation. 1999. Radiation security norms (RSN-99).
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Cleaning Up Sites Contaminated with Radioactive Materials: International Workshop Proceedings
TABLE 24-2 Numbers of Population Centers in the Russian Federation by Level of Cesium-137 Contamination on an Oblast or Autonomous Republic Basis (Conditions as of January 2006)
Oblast or Autonomous Republic
Total Population Centers
Total Samples
<1 Ci/km2
1-5 Ci/km2
5-15 Ci/km2
15-40 Ci/km2
>40 Ci/km2
Population Centers
Sample
Population Centers
Sample
Population Centers
Sample
Population Centers
Sample
Population Centers
Sample
Bashkortostan
16
65
16
65
Belgorod
550
3,597
419
3,007
131
590
Bryansk
2,007
25,419
1,313
11,589
428
4,676
212
6,764
51
2,301
3
747
Volgograd
5
24
4
17
1
5
Voronezh
1,208
9,636
1,136
8,901
72
735
Kaluga
591
5,952
325
2,250
242
3,220
24
400
Kursk
1,111
6,719
984
5,616
127
1,103
Leningrad
159
1,732
122
1,335
37
430
Lipetsk
214
1,607
170
1,281
44
375
Mary El
25
72
25
72
Mordovia
390
1,459
373
1,358
17
98
Moscow
9
49
9
49
Nizhny Novgorod
148
742
148
742
Novgorod
85
492
85
492
Oryol
1,596
11,850
1,001
7,201
594
4,640
1
9
Penza
202
1,483
180
1,335
22
119
Rostov
2
10
2
10
Ryazan
579
7,365
405
5,871
174
2,493
Saratov
11
41
11
41
Smolensk
89
513
89
513
Tambov
123
961
121
935
2
26
Tula
2,391
19,005
1,340
7,943
995
9,855
56
1,207
Ulyanovsk
131
559
130
552
1
4
Chuvashia
34
89
34
33
TOTAL
11,676
105,904
8,442
61,208
2,887
28,369
293
8,380
51
2,301
3
747
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Cleaning Up Sites Contaminated with Radioactive Materials: International Workshop Proceedings
TABLE 24-3 Year When Last Population Center in Each Area Listed in Table 24-2 Will Shift from One Cesium-137 Contamination Category to the Next Lower
Oblast or Autonomous Republic
1-5 Ci/km2
5-15 Ci/km2
15-40 Ci/km2
>40 Ci/km2
Belgorod
2048
Bryansk
2180
2110
2063
2020
Volgograd
2020
Voronezh
2044
Kaluga
2100
2030
Kursk
2050
Leningrad
2044
Lipetsk
2039
Mordovia
2040
Oryol
2077
2007
Penza
2050
Ryazan
2054
Tambov
2007
Tula
2109
2039
Ulyanovsk
2011
TOTAL
2180
2110
2063
2020
FIGURE 24-1 Changes in average annual cesium-137 activity by volume in the air over the city of Bryansk since the Chernobyl accident.
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Cleaning Up Sites Contaminated with Radioactive Materials: International Workshop Proceedings
FIGURE 24-2 Annual cesium-137 fallout at Krasnaya Gora settlement.
FIGURE 24-3 Cesium-137 concentrations in the soil in Krasnaya Gora settlement.
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Cleaning Up Sites Contaminated with Radioactive Materials: International Workshop Proceedings
TABLE 24-4 Concentrations of Cesium-137, Strontium-90, and Tritium in Surface Water and Well Water, 1998-1999
Body of Water
Concentration, Bq/L
Cs-137
Sr-90
Tritium
Lake Svyatoye na Besedi
11.1-11.4
0.40-0.42
1.6-2.1
Lake Kozhanovskoye
5.1-7.1
1.1-1.5
1.4-3.0
Outflow canal from Lake Kozhanovskoye
4.4-5.9
Nagorny Canal
0.5-1.4
Karyer Reservoir
0.30-0.34
0.57-0.86
2.1-3.1
Ponds in rural settlements Yalovka and Nikolaevka
0.6-5.4
0.37-0.91
1.8-2.8
Other small bodies of water
0.07-3.54
0.17-0.71
1.2-4.2
Rivers Iput, Besed, Snov, Korna, Vaga, Tsata
0.01-0.23
0.021-0.095
1.9-2.7
Wells in rural settlement Nikolaevka
0.05-0.4
Well in rural settlement Zaborye
0.08
Well in center of rural settlement Kozhany
0.03
1.5
Borehole in urbanized settlement Mirny, school, water pipeline
0.2
RSN-99 levels of intervention, Bq/L
11
5
7,700
The levels of radioactive contamination in bodies of water in Bryansk Oblast were also studied in detail.4 Some results of this research are presented in Table 24-4 and Figure 24-4. The table and figure show that levels of contamination in the water in rivers flowing through the contaminated areas of Bryansk Oblast and in wells located in the most contaminated population centers (Kozhany, Nikolaevka, and Zaborye) are two to three orders of magnitude below the level of intervention established by RSN-99. However, contamination levels in water in closed reservoirs located near those population centers (Lake Kozhanovskoye and Lake Svyatoye na Besedi) are close to or exceed the level of intervention. High levels of cesium-137 contamination in fish have also been identified in these lakes. Table 24-5 presents data on contamination levels in fish from these lakes. As shown in the table, the contamination levels in fish exceeded the maximum allowable level by one to two orders of magnitude.
4
Vakulovsky, S. M., et al. 2000. Radioecological monitoring of the environment in Bryansk Oblast in 1998-1999. Pp. 19-23 in Proceedings of the International Conference on Radioactivity Associated with Nuclear Explosions and Accidents, April 24-26, 2000, Moscow, vol. 2.
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Cleaning Up Sites Contaminated with Radioactive Materials: International Workshop Proceedings
FIGURE 24-4 Cesium-137 concentration in lakes Svyatoye and Kozhanovskoye.
TABLE 24-5 Specific Cesium-137 Activity Levels in Fish, 1998-1999
Fish
Length, cm
Body of Water
Specific Activity, kBq/kg dry weight
Cs-137 Bioconcentration Factor in Fish, L/kg
Perch
5
Zalomenye
0.6
1,600
Carp
10
Yalovka
0.3
400
Carp
21-23
Vereshchaki
0.3
400
Carp
21-26
Karyer
0.1-0.3
300-900
Carp
25-30
Kozhanovskoye
5.2-9.5
1,100-2,100
Carp
20-36
Kozhanovskoye
6.1-10.0
1,300-2,200
Ruffe
10
Karyer
0.13
400
Northern pike
66
Karyer
0.7
2,200
Northern pike
17-43
Kozhanovskoye
5.5-12.4
1,200-2,700
Roach
10-15
Kozhanovskoye
2-5.8
400-1,300
Roach
22
Kozhanovskoye
6
1,300