analyses of stellar nucleosynthesis. In stellar astrophysics, the debris from nuclear reactions inside a star is used to infer detailed information about the nature of the star and the reactions, including the mass, density, compositional layers, and temperature of the star. Very similar analyses are used in nuclear forensics to answer the pertinent questions for an exploded nuclear device here on Earth.
During the nuclear testing era, the United States and other countries used radiochemistry techniques to characterize the explosions from collected debris. The application of the radio-chemistry experience and techniques developed over those decades has proved invaluable in generating the key concepts underlying nuclear forensics. The current forensic capabilities have been used in postdetonation exercises in which the national laboratories have demonstrated that they can characterize nuclear debris and other forensic data and can infer the key design features for a variety of hypothesized nuclear explosive devices.
Several key nuclear physics concepts apply in forensics. One is the use of the natural radioactive decay of a nuclear material to determine its age. Plutonium, which does not occur naturally on Earth, would originally have been produced in a reactor with some unavoidable plutonium-240 and plutonium-241 content. The decay of plutonium-241 into americium-241 with a 14.4-year half-life indicates the time lapsed since production. This is analogous to the way in which carbon dating is used to determine the age of some material. Key information regarding the origin of plutonium material can also be obtained from the ratio of the different plutonium isotopes—for example, whether it is weapons grade or reactor grade and the total reactor neutron fluence (or burnup) to which it was originally exposed.
The design of a detonated device from the explosion debris can be inferred from the shape of the neutron flux spectrum, which serves as a fingerprint for the design. An analogous fingerprint for nuclear reactors is the average energy of the neutron spectrum, from which one can deduce whether the reactor is a thermal light or heavy water reactor or a fast reactor, which will point to whoever designed the reactor. To extract the shape of the neutron flux spectrum for a detonated nuclear device, forensics takes advantage of the very different energy dependencies of nuclear cross sections. Useful nuclear reactions fall into three categories: (1) neutron capture, which characterizes the low-energy part of the spectrum, (2) inelastic neutron scattering to nuclear isomers, which characterizes the fission neutron component of the spectrum, and (3) threshold (n, 2n) reactions, which characterize the high-energy component of the spectrum from fusion neutrons.
As an example, let us consider how we could use the americium-241 present in the fuel of a plutonium-based nuclear device to extract information about the shape of the neutron spectrum. During the explosion, some of the americium-241 will be transmuted to americium-240 through the (n,2n) reaction; this americium-240 could not have been present before detonation because it lives for only 2.1 days. Producing americium-240 from americium-241 requires the presence of neutrons with energies of at least 6.67 MeV, because the nuclear reaction involved is a so-called threshold reaction. Thus, the relative abundance of americium-240 provides unique information about the high-energy component of the neutron spectrum (see Figure FOR 2).
Detailed studies of the implication of the production of americium-240 or other isotopes of interest require that all of the significant paths for producing and destroying these isotopes during a nuclear explosion be known. To address this requirement, a number of multiinstitutional programs are performing a series of measurements. One of the collaborations is attempting the first measurement of the fission of americium-240, a very challenging undertaking for several reasons. The first two challenges are the production of a significant quantity of americium-240 and its subsequent chemical separation to form a target. These are being carried out at LBNL using the 88-in. cyclotron and radiochemistry facilities. Stewardship Science fellow Paul El-